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• W2079365038 abstract "Millimeter-sized “liquid marbles” are usually prepared using highly hydrophobic particles such as fluorosilane-treated lycopodium powder or alkylated silica sols. In the present work it is shown that “liquid marbles” can be prepared using sterically stabilized polystyrene latex; remarkably, such latex particles can be readily prepared by aqueous emulsion polymerization using a well-defined styrene-functionalized poly(2-(diethylamino)ethyl methacrylate) macromonomer as a reactive steric stabilizer. The macromonomer stabilizer chains are water-soluble when partially protonated below their pKa of ∼7.0 but become sufficiently hydrophobic in their deprotonated form to allow formation of robust “liquid marbles” that remain stable when placed at the air/water interface. Moreover, the stabilizer chains confer pH-responsive behavior on the “liquid marbles”; addition of acid to the aqueous subphase causes immediate destruction of the “liquid marble”." @default.
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• W2079365038 date "2009-03-31" @default.
• W2079365038 modified "2023-10-06" @default.
• W2079365038 title "Stimulus-Responsive Liquid Marbles" @default.
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• W2079365038 doi "https://doi.org/10.1021/ja901641v" @default.
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