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• W2079380092 abstract "Recent advances in the synthesis of multicomponent nanocrystals have enabled the design of nanocrystal molecules with unique photophysical behavior and functionality. Here we demonstrate a highly luminescent nanocrystal molecule, the CdSe/CdS core/shell tetrapod, which is designed to have weak vibronic coupling between excited states and thereby violates Kasha's rule via emission from multiple excited levels. Using single particle photoluminescence spectroscopy, we show that in addition to the expected LUMO to HOMO radiative transition, a higher energy transition is allowed via spatially indirect recombination. The oscillator strength of this transition can be experimentally controlled, enabling control over carrier behavior and localization at the nanoscale." @default.
• W2079380092 created "2016-06-24" @default.
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• W2079380092 date "2011-05-19" @default.
• W2079380092 modified "2023-10-09" @default.
• W2079380092 title "Spatially Indirect Emission in a Luminescent Nanocrystal Molecule" @default.
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• W2079380092 doi "https://doi.org/10.1021/nl2007032" @default.
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• W2079380092 hasPublicationYear "2011" @default.
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