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- W2079475450 abstract "X-ray structure factors for heavy water were measured at temperatures of 40.0, 23.5, 15.5, 11.2, 7.1, 0.2, and -11.0ifmmode^circelsetextdegreefi{}C. From these data isochoric temperature differentials (ITD) were constructed for pairs of temperatures $ensuremath{Delta}T=40.0ensuremath{-}(ensuremath{-}11.0)=51.0,23.5ensuremath{-}0.2=23.3,mathrm{and} 15.5ensuremath{-}7.1=8.4$ ifmmode^circelsetextdegreefi{}C around the maximum density point at 11.2ifmmode^circelsetextdegreefi{}C. We show that the temperature dependence of the structural parameters can be obtained much more precisely from ITD than from the direct determination of the structure factor. A major structural rearrangement at the second-neighbor shell is identified from the interpretation of the ITD. We then interpret this rearrangement in terms of a possible increased molecular angular correlation of the tetrahedral structure at low temperatures." @default.
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- W2079475450 date "1983-03-01" @default.
- W2079475450 modified "2023-10-18" @default.
- W2079475450 title "Isochoric temperature differential of the x-ray structure factor and structural rearrangements in low-temperature heavy water" @default.
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- W2079475450 doi "https://doi.org/10.1103/physreva.27.1468" @default.
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