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- W2079556614 abstract "Abstract Using the Optical Stochastic Bloch equations (OSBE), and considering a two-level molecular system interacting with a thermal reservoir (modeled as an Ornstein–Uhlenbeck process) in four-wave mixing spectroscopy, we derive analytical expressions for the nonlinear optical properties (absorptive and dispersive processes). Here, we have widened the previous formalism [(J.L. Paz et al., Phys. Lett. A 226 (1997) 365)] to consider the solvent effects and high-pump-power in the four-wave mixing (FWM) technique. The saturation effects introduced by including high-pump-power are explicitly considered. These results are very useful when laser-beams of moderate or high-intensity are employed for the determination of relaxation mechanisms in molecular systems interacting explicitly with their environment." @default.
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- W2079556614 date "1999-12-01" @default.
- W2079556614 modified "2023-10-01" @default.
- W2079556614 title "Analysis of the stochastic effects of the solvent and high-pump-power on the nonlinear optical properties in four-wave mixing spectroscopy" @default.
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- W2079556614 doi "https://doi.org/10.1016/s0166-1280(99)00240-7" @default.
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