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- W2079557325 abstract "In order to elucidate the magnetism and Li diffusion in LiFePO${}_{4}$, we have measured muon-spin rotation and relaxation (${ensuremath{mu}}^{+}$SR) spectra for the polycrystalline LiFePO${}_{4}$ sample in the temperature range between 1.8 and 500 K. Below ${T}_{mathrm{N}}ensuremath{sim}52$ K, two oscillatory signals together with one fast relaxation signal were clearly found in the zero-field (ZF) ${ensuremath{mu}}^{+}$SR spectrum. The three signals are reasonably explained using an antiferromagnetic (AF) spin structure proposed by neutron measurements, because electrostatic potential calculations suggests multiple different muon sites in the LiFePO${}_{4}$ lattice. However, the AF ordered moment estimated from ${ensuremath{mu}}^{+}$SR was about 3/4 of that reported by neutron, probably due to a different time window between the two techniques. In the paramagnetic state, ZF and longitudinal-field (LF) ${ensuremath{mu}}^{+}$SR spectra exhibited a dynamic nuclear field relaxation. From the temperature dependence of the field fluctuation rate, a diffusion coefficient of Li${}^{+}$ ions (${D}_{mathit{Li}}$) at 300 K was estimated about $3.6ifmmodetimeselsetexttimesfi{}{10}^{ensuremath{-}10}$ cm${}^{2}$/s, assuming that diffusing Li${}^{+}$ ions jump between the regular site and interstitial sites." @default.
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- W2079557325 date "2011-08-09" @default.
- W2079557325 modified "2023-10-04" @default.
- W2079557325 title "Magnetic and diffusive nature of LiFePO<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:msub><mml:mrow /><mml:mn>4</mml:mn></mml:msub></mml:math>investigated by muon spin rotation and relaxation" @default.
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- W2079557325 doi "https://doi.org/10.1103/physrevb.84.054430" @default.
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