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• W2079603417 abstract "Si is a promising anode material for Li-ion batteries, since it absorbs large amounts of Li. However, insertion of Li leads to 334% of volumetric expansion, huge stresses, and fracture; it can be suppressed by utilizing nanoscale anode structures. Continuum approaches to stress relaxation in LixSi, based on plasticity theory, are unrealistic, because the yield strength of LixSi is much higher than the generated stresses. Here, we suggest that stress relaxation is due to anisotropic (tensorial) compositional straining that occurs during insertion-extraction at any deviatoric stresses. Developed theory describes known experimental and atomistic simulation data. A method to reduce stresses is predicted and confirmed by known experiments. Chemical potential has an additional contribution due to deviatoric stresses, which leads to increases in the driving force both for insertion and extraction. The results have conceptual and general character and are applicable to any material systems." @default.
• W2079603417 created "2016-06-24" @default.
• W2079603417 creator A5003738174 @default.
• W2079603417 creator A5076056522 @default.
• W2079603417 date "2013-04-08" @default.
• W2079603417 modified "2023-09-24" @default.
• W2079603417 title "Anisotropic Compositional Expansion and Chemical Potential for Amorphous Lithiated Silicon under Stress Tensor" @default.
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• W2079603417 doi "https://doi.org/10.1038/srep01615" @default.
• W2079603417 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/3619142" @default.
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• W2079603417 hasPublicationYear "2013" @default.
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