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- W2079631566 abstract "Chiral surfaces, capable of existing in two distinguishable mirror forms that cannot be superimposed, are attracting worldwide attention. The adsorption of complex organic molecules provides a means of introducing the ultimate discrimination function of chirality to a metal surface. Here, a comparison of the chiral tartaric acid (HOOC–CHOH–CHOH–COOH) molecule and the achiral succinic acid (HOOC–CH2–CH2–COOH) molecule on a Cu(110) surface is presented. For both molecules, two-dimensional assembly is found to depend strongly on molecule–metal bonding interactions, whereas the presence/absence of the OH groups causes subtler, second-order effects on the self-assembled structure. The driving force for creating chiral organisations is shown to arise from adsorption-induced asymmetrisation, via molecular distortion and/or metal reconstruction of the local adsorption unit. The macroscopic chirality of the surface is then determined by whether nucleation points of both chirality can be equally created, or whether non-degeneracy can be introduced to favour one chirality." @default.
- W2079631566 created "2016-06-24" @default.
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- W2079631566 date "2005-02-01" @default.
- W2079631566 modified "2023-10-17" @default.
- W2079631566 title "Chiral metal surfaces from the adsorption of chiral and achiral molecules" @default.
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- W2079631566 doi "https://doi.org/10.1016/j.apsusc.2004.09.058" @default.
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