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- W2079662571 startingPage "2301" @default.
- W2079662571 abstract "An investigation of nuclear spin lattice relaxation was performed on a conductive Langmuir-Blodgett (LB) film based on a charge-transfer (CT) complex of bisethylenedioxytetrathiafulvalene (BO) and decyltetracyanoquinodimethane $({mathrm{C}}_{10}mathrm{TCNQ}).$ The characteristic peak of the relaxation rate ${T}_{1}^{ensuremath{-}1}$ of ${}^{1}mathrm{H}$ was observed at a low temperature (10 K). As in its pristine solid $(mathrm{BO}ensuremath{-}{mathrm{C}}_{10}mathrm{TCNQ}$ complex), the behavior of the relaxation rate was explained by the theory of localization. From the quantitative analysis of the behavior, the detailed dynamics of the localized electrons in the LB film were successfully obtained. In addition, the outer-planar anisotropy of ${T}_{1}^{ensuremath{-}1}$ of ${}^{1}mathrm{H}$ was observed in the LB film. This indicates that the observed echo mainly originated from ${}^{1}mathrm{H}$ at the end ethylene groups of BO. The fact that the field dependence of this anisotropic ${T}_{1}^{ensuremath{-}1}$ is well fitted by the cosine curve provides detailed information of the hyperfine structures in the LB film. Considering these results in combination with those of the temperature dependence of ${T}_{1}^{ensuremath{-}1},$ it is concluded that the variance of each level of BO is small and that the nature of disorder in the LB film is that of a continuum." @default.
- W2079662571 created "2016-06-24" @default.
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- W2079662571 date "1999-01-15" @default.
- W2079662571 modified "2023-10-16" @default.
- W2079662571 title "NMR study of localized electrons in conductive Langmuir-Blodgett films" @default.
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- W2079662571 doi "https://doi.org/10.1103/physrevb.59.2301" @default.
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