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- W2079736360 abstract "Auger-electron-photoion coincidence (AEPICO) studies of photon-stimulated ion desorption (PSID) for condensed acetonitrile induced by carbon core excitation have been performed to elucidate the desorption mechanism related to the Auger process. We have detected only the H+ ion in AEPICO spectra. The total ion yield spectrum divided by the total electron yield shows that the desorption efficiency is largely increased at the resonant excitation to CH∗. We have also measured the Auger electron spectrum and the AEPICO yield spectrum at the CH∗ excitation. The AEPICO yield spectrum shows enhancement at 245–250 eV electron energy. This seems to be related to the spectator resonant Auger stimulated ion desorption. That is, H+ desorption is enhanced due to a two-hole-one-electron state at which the electron is in an anti-bonding CH∗ orbital and the two holes can be in a 1π bonding orbital localized on the CH3 group. We have also measured similar spectra for other resonant excitation (π∗CN, σ∗CC, σ∗CN). The results are discussed in connection with the bonding/anti-bonding character and localized character of the excited state." @default.
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- W2079736360 date "1997-11-01" @default.
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- W2079736360 title "Auger-electron-ion coincidence study of photon-stimulated ion desorption for condensed acetonitrile" @default.
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- W2079736360 doi "https://doi.org/10.1016/s0039-6028(97)00526-8" @default.
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