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- W2079774570 abstract "The syntheses and spectroscopic characterization of two 1,2,4-triazole-based oxovanadium(V) complexes are reported: 1- [VO2L1]- and 2 [(VOL2)2(OMe)2] (where H2L1 = 3-(2'-hydroxyphenyl)-5-(pyridin-2' '-yl)-1H-1,2,4-triazole, H3L2 = bis-3,5-(2'-hydroxyphenyl)-1H-1,2,4-triazole). The ligand environment (N,N,O vs O,N,O) is found to have a profound influence on the properties and reactivity of the complexes formed. The presence of the triazolato ligand allows for pH tuning of the spectroscopic and electrochemical properties, as well as the interaction and stability of the complexes in the presence of hydrogen peroxide. The vanadium(IV) oxidation states were generated electrochemically and characterized by UV-vis and EPR spectroscopies. For 2, under acidic conditions, rapid exchange of the methoxide ligands with solvent [in particular, in the vanadium(IV) redox state] was observed." @default.
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- W2079774570 date "2006-03-04" @default.
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- W2079774570 title "Electronic Properties, Redox Behavior, and Interactions with H<sub>2</sub>O<sub>2</sub> of pH-Sensitive Hydroxyphenyl-1,2,4-triazole-Based Oxovanadium(V) Complexes" @default.
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- W2079774570 doi "https://doi.org/10.1021/ic051848x" @default.
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