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• W2079842069 abstract "Abstraction of H adsorbed on Pt(111) surfaces by gaseous D atoms was studied with direct product detection as a function of coverage and atom flux at a substrate temperature of 85 K. The reaction products are HD and the homonuclear surface species H2. The product reaction kinetics is very similar to that of the alternate isotope combination, H→Dad, reported earlier. The reaction kinetics is not in accordance with the operation of an Eley–Rideal mechanism but is better described by a hot atom scheme. With both isotope combinations the kinetics is independent of the atom flux. The reaction yield of the homonuclear species scales with the square of the species' initial coverage, in accordance with a second-order process as origin of these products. Isotope effects were not observed in the yields, but were apparent in abstraction cross-sections." @default.
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• W2079842069 date "1998-08-01" @default.
• W2079842069 modified "2023-10-14" @default.
• W2079842069 title "Abstraction of H adsorbed on Pt(111) surfaces with gaseous D atoms: isotope and flux effects" @default.
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• W2079842069 doi "https://doi.org/10.1016/s0039-6028(98)00326-4" @default.
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