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• W2079869619 abstract "• Fe-CN/TS-1 hybrid materials are fabricated by a facial thermal polymerization approach using dicyandiamide, metal chloride as precursors and TS-1 zeolite as a support. • In contrast with pure TS-1, the photocurrent of the as-synthesized Fe-CN/TS-1 composites improves evidently. • Compared with pure Fe-CN and TS-1 catalyst, the as-synthesized Fe-CN/TS-1 composite displays improved photocatalytic activities (9 and 4 times, respectively) for the phenol production from benzene with H 2 O 2 under mild conditions. Fe-g-C 3 N 4 (denoted as Fe-CN) and titanium silicate zeolite (TS-1) hybrid materials were fabricated by a facial thermal polymerization approach using dicyandiamide, metal chloride as precursors and TS-1 zeolite as a support. The structure and textural properties of the resulting hybrid materials were thoroughly characterized by X-ray diffraction, UV–Vis spectrophotometry, nitrogen adsorption–desorption isotherm, Fourier transform infrared spectroscopy, scanning transmission electron microscopy, X-ray photoelectron spectroscopy and electrochemical measurement. The as-synthesized Fe-CN/TS-1 composites could be used as heterogeneous catalysts for the photocatalytic selective oxidation of benzene to phenol using H 2 O 2 as benign oxidant under ambient conditions. It is found that the Fe-CN/TS-1 hybrid materials show superior photocatalytic performance for the phenol production from benzene to sole Fe-CN and TS-1 catalysts. Under the optimal conditions, up to 10.0% phenol yield (based on benzene) is achieved over the hybrid materials, with 18.4% phenol selectivity (based on H 2 O 2 )." @default.
• W2079869619 created "2016-06-24" @default.
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• W2079869619 date "2014-06-01" @default.
• W2079869619 modified "2023-10-16" @default.
• W2079869619 title "Selective oxidation of benzene to phenol by Fe-CN/TS-1 catalysts under visible light irradiation" @default.
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• W2079869619 doi "https://doi.org/10.1016/j.apcatb.2014.01.050" @default.
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