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• W2079959501 abstract "We present phase diagrams of binary blends (or mixtures) of a homopolymer H, with a block copolymer, A—B, in which there is an exothermic interaction between two types of segments, H and A. In trying to construct phase diagrams, we extend the approach of predicting phase separation behaviour in such binary blends where H is chemically identical with one of the blocks of the copolymer, e.g. A. A binary blend of a homopolymer with a block copolymer is divided into two distinct states, i.e. an ordered state and a disordered state. On the assumption that the block copolymer in the disordered state acts as a random copolymer, the free-energy change in the disordered state can be estimated by a model including the localized solubilization of added homopolymers, which is a modification of the confined-chain model originated by Meier. To determine coexisting phases under a given temperature, we examine the relative stabilities (i.e. the chemical potential of each component in the blend) of the two states. As a result, the concentration—temperature phase diagrams of blends of H and A-B can be obtained. From the predicted phase diagrams, it is found that the exothermic interaction of this system greatly increases the solubility of H into the A domains and affects the shape of the phase diagram." @default.
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• W2079959501 date "1996-01-01" @default.
• W2079959501 modified "2023-10-13" @default.
• W2079959501 title "Phase diagrams for block copolymer/ homopolymer blends exhibiting LCST behaviour" @default.
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• W2079959501 doi "https://doi.org/10.1016/0032-3861(96)81101-3" @default.
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