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- W2080257456 abstract "A kinetic analysis of ammonia synthesis over powdered Co showed that the rate law is of the type r = kPN2(1 + KPH212)−2(1 + K′PNH3)−2 The reaction was rate limited by N2 chemisorption and inhibited, albeit moderately, by H2 and NH3. Within the temperature domain where the reaction could be studied, Co underwent the hcp ⇌ fcc phase transformation. Little variation of the active area was entailed but a significant change was observed for the rate constant of N2 chemisorption, the equilibrium constant of H2 chemisorption and also the equilibrium constant of chemisorbed nitrogen. Every step (or group of steps) of the reaction was therefore involved, leading to a variation of the overall rate of reaction. Another striking effect of the phase transformation was the display of reversible hysteresis cycles as a function of the temperature." @default.
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- W2080257456 date "1985-07-01" @default.
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- W2080257456 title "Catalytic activity of a cobalt powder in NH3 synthesis in relation with the allotropic transformation of the metal" @default.
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- W2080257456 doi "https://doi.org/10.1016/0021-9517(85)90091-0" @default.
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