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- W2080321279 abstract "The density-matrix approach, in the quasistatic or adiabatic limit, is applied to the case of resonant four-wave interactions in four-level systems resulting in explicit analytical expressions for the nonlinear optical parametric and nonparametric polarizations, including ac Stark effects. The results are applicable to any closed-linkage diagram of this type but are applied only to the specific case of resonant frequency tripling. The results revealed the presence of up to six Stark-shifted nonparametric resonances and the presence of saturation and interference effects on the parametric susceptibility. In particular, the third-order susceptibility is shown to saturate to a very small value under high-field conditions which restricts the range of useful pump intensities. Under near-resonant to resonant conditions, these imply that because of either nonparametric loss present at the pump or harmonic frequencies or power-dependent dispersive and saturation effects, conversion efficiencies higher than 25% may be difficult to realize in practice." @default.
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- W2080321279 date "1988-05-01" @default.
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- W2080321279 title "Resonant four-wave parametric interactions: Adiabatic formulation" @default.
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- W2080321279 doi "https://doi.org/10.1103/physreva.37.3358" @default.
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