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- W2080334189 abstract "The magnetism of $mathrm{Pt}$-rich $mathrm{Pt}text{ensuremath{-}}mathrm{Mn}$ alloys was studied in single crystals with different $mathrm{Mn}$ concentrations (12.5, 14.4, and $15.9phantom{rule{0.3em}{0ex}}text{at}mathrm{.}%$) and different atomic arrangements of disordered, ${mathrm{ABC}}_{6}$ type and ${mathrm{Cu}}_{3}mathrm{Au}$ type structures by using neutron scattering and susceptibility measurements. The neutron scattering measurements showed drastic changes in the magnetic diffraction pattern with a slight difference in the atomic arrangement and $mathrm{Mn}$ concentration. In disordered alloys, magnetic diffuse peaks were observed at $1∕2$, 0, 0 and equivalent symmetry positions of the fcc fundamental structure. In ordered alloys with the ${mathrm{ABC}}_{6}$ type structure, fourfold splitting along $[011]$ and $[0overline{1}1]$ with incommensurate maxima appeared in the $1∕2$, 0, 0 diffuse scattering in $mathrm{Pt}text{ensuremath{-}}12.5phantom{rule{0.3em}{0ex}}text{at.}%mathrm{Mn}$, while the $1∕2$, 0, 0 diffuse scattering completely disappeared, instead, commensurate superlattice peaks were newly observed at $1∕2,ifmmodepmelsetextpmfi{}1∕4,0$ and $1∕2,0,ifmmodepmelsetextpmfi{}1∕4$ in $mathrm{Pt}text{ensuremath{-}}14.4phantom{rule{0.3em}{0ex}}text{at.}%mathrm{Mn}$. Fourfold splitting and superlattice peaks were observed with the ${mathrm{ABC}}_{6}$ type symmetry. In ordered alloys with the ${mathrm{Cu}}_{3}mathrm{Au}$ type structure, ferromagnetic diffuse scattering was mainly observed at the zone center of the ${mathrm{Cu}}_{3}mathrm{Au}$ type structure. The origin of these magnetic scatterings is discussed in terms of three different magnetic interactions: a spin-density wave (SDW) originated by a nesting Fermi surface, an antiferromagnetic interaction on the ${mathrm{ABC}}_{6}$ type structure and a ferromagnetic interaction on the ${mathrm{Cu}}_{3}mathrm{Au}$ type structure. The dominant interaction largely depends on the atomic arrangement, indicating a strong coupling between the magnetic and atomic structures in the alloys. Susceptibility measurements showed a spin-glass-like behavior in all of the samples, which is attributed to the dynamics of the fluctuating SDW clusters, as observed in other $mathrm{Pd}text{ensuremath{-}}mathrm{M}$ and $mathrm{Pt}text{ensuremath{-}}mathrm{M}$ ($mathrm{M}$; $3d$ element) spin-glass alloys. The persistence of the SDW fluctuations indicates the instability of these magnetic structures." @default.
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- W2080334189 date "2004-07-29" @default.
- W2080334189 modified "2023-10-18" @default.
- W2080334189 title "Magnetic structures and spin-glass-like behavior in ordered and disorderedPt-richPt−Mnalloys" @default.
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- W2080334189 doi "https://doi.org/10.1103/physrevb.70.014431" @default.
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