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- W2080346501 abstract "Abstract A series of supported Ni/TiO 2 catalysts were prepared by incipient wetness impregnation method under different calcination temperatures, and the as-prepared catalysts were characterized by X-ray diffraction (XRD), hydrogen temperature-programmed reduction (H 2 -TPR) and X-ray photoelectron spectroscopy (XPS). The catalytic properties of these Ni/TiO 2 catalysts were investigated in the vapor phase hydrogenation of maleic anhydride (MA) to succinic anhydride (SA). The results showed that the catalytic activity and the selectivity of the Ni/TiO 2 catalysts were strongly affected by the calcination temperature. The catalyst calcined at 1023 K showed a relatively higher SA selectivity of 96% at high MA conversion (96%) under the tested conditions (493 K and 0.2 MPa). The improvement of SA selectivity could be mainly assigned to the presence of suitable metal–support interaction, which can play a role in catalytic property of active nickel species as electron promoter. Besides, the change of surface properties of TiO 2 support with the increasing calcination temperatures, e.g., the decrease of Lewis acid sites, might also have some positive role in reducing the side-products like γ-butyrolacetone (GBL)." @default.
- W2080346501 created "2016-06-24" @default.
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- W2080346501 date "2014-11-01" @default.
- W2080346501 modified "2023-10-11" @default.
- W2080346501 title "Vapor-phase selective hydrogenation of maleic anhydride to succinic anhydride over Ni/TiO2 catalysts" @default.
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- W2080346501 doi "https://doi.org/10.1016/j.jiec.2014.01.012" @default.
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