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• W2080441025 abstract "ABSTRACT Chemisorbed films of octadecyltrichlorosilane (OTS) and ethyltrichiorosilane (ETS) at the interface calcium fiuo-ride:air have been studied by vibrationally resonant JR pump JR-vis probe sum-frequency (SF) spectroscopy. Usinga total internal reflection geometry, a signal enhancement of more than two orders of magnitude compared to theconventional setup is achieved. This enhancement in combination with two independently continously tunable in- frared sources provide new insight in intramolecular energy flow processes and the corresponding relaxation times on dielectric surfaces. A fast energy exchange between the CH3-stretching modes detected by SF spectroscopy occurs within a few picoseconds. A two-exponential decay of the CH3-stretching modes is observed: The energy relaxation is fast with time constants in the picosecond range, while the ground state is repopulated in approximately 100 Ps. Due to the fast energy exchange within the CH-stretching vibrations and their strong anharmonic coupling, bleaching" @default.
• W2080441025 created "2016-06-24" @default.
• W2080441025 creator A5037050218 @default.
• W2080441025 creator A5060126980 @default.
• W2080441025 date "1998-12-30" @default.
• W2080441025 modified "2023-09-23" @default.
• W2080441025 title "<title>Surface studies using nonlinear spectroscopy with tunable picosecond pulses</title>" @default.
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• W2080441025 doi "https://doi.org/10.1117/12.334804" @default.
• W2080441025 hasPublicationYear "1998" @default.
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