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• W2080450194 abstract "A mixed zirconium–lanthanum phosphate La1/3Zr2(PO4)3, noted LaZrP, is studied as a potential host for actinides issued from high-level nuclear wastes. Chemical durability is evaluated and compared with two other phases: a monazite phase LaPO4, noted LaP, and a mixed oxide phase La0.1ZrO2.15, noted LaZrO. Leaching tests are performed and followed by solution and solid analyses. Static tests are performed with a low ratio between surface of ceramic and volume of solution, S/V (about 0.1cm−1). For LaZrP, the phosphate release rate decreases from 10−2 to 10−3g/m2/day, while zirconium and lanthanum releases remain very low (<10−5g/m2/day). For the LaP phase, the phosphate release is about 10 times lower than for LaZrP and remains stationary, while the rate of the lanthanum release is below 10−6g/m2/day. Tests performed at high S/V (about 20cm−1) reveal that the lanthanum release rates after 2 weeks were, respectively, at 10−9, 10−6 and 10−4g/m2/day for LaP, LaZrP and LaZrO phases. It is shown that NZP or monazite type ceramics are highly resistant to the leaching process." @default.
• W2080450194 created "2016-06-24" @default.
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• W2080450194 date "2001-08-01" @default.
• W2080450194 modified "2023-09-25" @default.
• W2080450194 title "Preliminary results on the leaching process of phosphate ceramics, potential hosts for actinide immobilization" @default.
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• W2080450194 doi "https://doi.org/10.1016/s0022-3115(01)00607-9" @default.
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