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- W2080479383 abstract "A systematic study of the broadening of the C 1s and O 1s 2ensuremath{pi} resonances for CO adsorbed in different ordered phases on Ni(100), Pd(100), and Cu(100), and for CO on Ag(110) is presented. The systems span a number of different adsorption energies and adsorption sites, as well as different adsorbate-adsorbate distances. The widths of the 2ensuremath{pi} resonances are found to be larger for strongly bonded and highly coordinated adsorbates but they are independent of the adsorbate-adsorbate separation. The broadening is larger for the O 1s than the C 1s 2ensuremath{pi} resonances and it increases with the final-state chemisorption energy. For weakly chemisorbed final states, the 2ensuremath{pi} width is dominated by vibrational excitations, while the adsorbate-substrate hybridization of the final core excited state determines the width in the case of strong chemisorption. Low-energy vibrational modes, like frustrated translations which are important for the broadening of adsorbate core-level photoelectron spectra, do not give any dominating contribution to the 2ensuremath{pi}-resonance broadening." @default.
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- W2080479383 date "1992-10-15" @default.
- W2080479383 modified "2023-10-16" @default.
- W2080479383 title "2π-resonance broadening in x-ray-absorption spectroscopy of adsorbed CO" @default.
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- W2080479383 doi "https://doi.org/10.1103/physrevb.46.10353" @default.
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