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- W2080497064 abstract "The proton spin—lattice relaxation time T1 has been measured by a pulse technique as a function of temperature in a series of tantalum-hydrogen samples with hydrogen content from H/Ta=0.1 to 0.66. The spin—lattice relaxation is determined by the rapid translational diffusion of the hydrogen atoms in the tantalum lattice. Discontinuities in the T1 curves indicate two phase transitions in the temperature range investigated, 200° to 400°K. The transition temperatures depend on the composition of the sample in a way which is in conflict with the present view of the phase relations in the Ta/H system. The activation energy in the low-temperature phase (β1 phase) is found to decrease linearly with increasing hydrogen content from 3.7±0.5 kcal/mole in TaH0.10 to 2.6±0.3 kcal/mole in TaH0.66. In the high-temperature phase (α phase) the activation energy is 1.6±0.4 kcal/mole, and in the intermediate-temperature phase (β2 phase) the activation energy is 6.3±0.6 kcal/mole. Neither of the latter values changes significantly with the composition of the sample." @default.
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- W2080497064 date "1965-01-01" @default.
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- W2080497064 title "On the Motion of Hydrogen in the Tantalum—Hydrogen System" @default.
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- W2080497064 doi "https://doi.org/10.1063/1.1695728" @default.
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