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- W2080592388 abstract "We discuss here the intercollisional memory effects which have been detected in the low-frequency region of the absorption spectra induced by collisions in dilute solutions of para-${mathrm{H}}_{2}$, He, and Ne in liquid argon. The theories of gaseous mixtures are shown to be inadequate to describe the spectra in liquids. Then we calculate the low-frequency part of the translational absorption spectrum for an argon crystal doped with impurities. The results of such a calculation for the solid are compared with the experimental data on liquid solutions and with the behavior predicted by the gaseous theories. We also show that from the induced-dipole-moment autocorrelation function, as obtained from the experimental data, it is possible to determine the short-time behavior of the force and velocity-autocorrelation functions of the impurity in the liquid. In particular we obtain the mean-square force $〈{F}^{2}〉$ acting on the impurity and $〈{stackrel{ifmmode dot{}else .{}fi{}}{F}}^{2}〉$. The derived values of $〈{F}^{2}〉$ and $〈{stackrel{ifmmode dot{}else .{}fi{}}{F}}^{2}〉$ are compared with those estimated with the help of the radial-distribution function of the liquid mixtures." @default.
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- W2080592388 date "1974-09-01" @default.
- W2080592388 modified "2023-10-16" @default.
- W2080592388 title "Intercollisional memory effects and short-time behavior of the velocity-autocorrelation function from translational spectra of liquid mixtures" @default.
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- W2080592388 doi "https://doi.org/10.1103/physreva.10.913" @default.
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