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• W2080684568 abstract "Using a coated-wall flow tube connected to a mass spectrometer, the heterogeneous conversion of NO2 to HONO on dry hydrocarbon soot surfaces has been studied at room temperature and 243 K. Particular attention was given to the measurement of the HONO yield as a function of hydrocarbon fuel, NO2 partial pressure, extent of uptake, and surface oxidation state. In all cases, the yield is invariant of these parameters and close to unity, indicative of an irreversible oxidation mechanism by which the NO2 abstracts an H atom from the surface. XPS analysis shows that the surface N content does not measurably increase with NO2 exposure. There is minimal surface reactivity regeneration with time or via exposure to high relative humidity. A BET surface area measurement of the entire soot film exposed to NO2 was used to determine the amount of HONO that can be generated from the soot surface per unit surface area, prior to its deactivation. The reduction of NO2 to HONO on soot is unlikely to account for the observed nighttime buildup of HONO in polluted urban environments." @default.
• W2080684568 created "2016-06-24" @default.
• W2080684568 creator A5010178344 @default.
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• W2080684568 date "2007-06-27" @default.
• W2080684568 modified "2023-10-16" @default.
• W2080684568 title "Interaction of NO₂ with Hydrocarbon Soot: Focus on HONO Yield, Surface Modification, and Mechanism" @default.
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• W2080684568 doi "https://doi.org/10.1021/jp068884h" @default.
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