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• W2080706153 abstract "Second harmonic generation (SHG) and angle-resolved absorbance with photoacoustic detection were combined to evaluate both the mean orientation angle and the width of the angular distribution for two surface-bound molecular systems. Assuming a Gaussian distribution function, a physisorbed stilbene dye on fused silica exhibited a narrow distribution centered at 73° with a root-mean-square (rms) width of less than ∼8°. In contrast, a covalently bound azo dye resulted in a broad orientation distribution (rms width of ∼30°) centered at 60°. It was also demonstrated that the combination of nonlinear (SHG) and linear (absorbance) spectroscopic techniques provides valuable insight into molecular orientation that a combination of two linear techniques (such as fluorescence and absorbance) is unable to provide." @default.
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• W2080706153 date "2000-02-01" @default.
• W2080706153 modified "2023-09-27" @default.
• W2080706153 title "Molecular Orientation and Angular Distribution Probed by Angle-Resolved Absorbance and Second Harmonic Generation" @default.
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• W2080706153 doi "https://doi.org/10.1021/ac9912956" @default.
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