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- W2080746670 abstract "Abstract The local atomic configurations measured from diffuse X-ray scattering in the gold-nickel system cannot be reconciled with the observed heats and entropies of mixing on the basis of a statistical treatment of chemical bonding energies. The heats of mixing are positive (heat absorbed), and yet there is a preference for unlike neighbours in solutions above the solubility gap. It is shown that these positive heats of mixing may be explained in terms of the elastic strain energy required to form solutions from atoms of different size. The sizes of the ions in gold-nickel solutions, also measured from the diffuse X-ray measurements, are used to calculate the strain energies and reasonable agreement with the observed heats of mixing is obtained. The strain energy contribution to the heat of mixing in Cu3Au is also evaluated approximately from an X-ray determination of the atomic size effect; in this system it appears that a significant negative contribution to the heat of mixing may arise from a change in the electronic configuration on alloy formation." @default.
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- W2080746670 date "1954-01-01" @default.
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- W2080746670 title "Solid solution formation in the gold-nickel system" @default.
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- W2080746670 doi "https://doi.org/10.1016/0001-6160(54)90099-1" @default.
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