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• W2080821278 abstract "We investigate the reaction kinetics of ultrafast excited state intramolecular proton transfer (ESIPT) and discuss the possible origins of the process: tunneling of the reactive proton, vibrationally enhanced tunneling, and multidimensional wave packet dynamics of the entire system. Comparison of the measured kinetics for the protonated and the deuterated form of 2-(2′-hydroxyphenyl)benzothiazole (HBT) to numerical simulations allows us to ascribe the characteristic 50 fs time found for the ESIPT solely to a ballistic wave packet motion along skeletal coordinates that mainly affect the donor acceptor distance. Tunneling is not found to be decisive." @default.
• W2080821278 created "2016-06-24" @default.
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• W2080821278 date "2011-02-01" @default.
• W2080821278 modified "2023-09-30" @default.
• W2080821278 title "The origin of ultrafast proton transfer: Multidimensional wave packet motion vs. tunneling" @default.
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• W2080821278 doi "https://doi.org/10.1016/j.cplett.2010.12.087" @default.
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