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• W2080855084 abstract "Relaxation dynamics of even parity ( ${A}_{g}$) states in poly( $p$-phenylene vinylene) derivatives are studied using a novel fsec transient spectroscopy, in which two different excitation pulses successively generate odd parity ( $1^{1}B_{u}$) excitons at 2.2 eV and then reexcite them to higher ${A}_{g}$ states. For reexcitation energies $ensuremath{Elzxh}ensuremath{omega}<1.1mathrm{eV}$ ultrafast internal conversion back to $1^{1}B_{u}$ takes place in accordance with Vavilov-Kasha's rule. However, for $ensuremath{Elzxh}ensuremath{omega}>1.1mathrm{eV}$ the decay occurs in a nonemissive state identified as a polaron pair, showing that the ${A}_{g}$ states above 3.3 eV mediate charge transfer." @default.
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• W2080855084 date "2000-09-04" @default.
• W2080855084 modified "2023-09-23" @default.
• W2080855084 title "Ultrafast Spectroscopy of Even-Parity States in<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mi>π</mml:mi></mml:math>-Conjugated Polymers" @default.
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• W2080855084 doi "https://doi.org/10.1103/physrevlett.85.2196" @default.
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