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• W2080883335 abstract "A hydrogen-bonded complex composed of the OH and CO reactants has been identified along the OH + CO-->HOCO reaction pathway. IR action spectroscopy in the OH overtone region has been used to examine the vibrational modes of the linear OH-CO complex, including intermolecular bending modes that probe portions of the reaction path leading to HOCO. The spectroscopic measurements have accessed highly excited intermolecular levels, with energies up to 250 cm-1 above the zero-point level, which lie in close proximity to the transition state for reaction. The OH-CO binding energy, D0 < or = 430 cm-1, has also been established from the quantum state distribution of the OH fragments following vibrational predissociation of the OH-CO complex. Complementary electronic structure calculations have been performed to characterize the OH-CO and OH-OC complexes, the transition state for HOCO formation, and the direct reaction path that connects the experimentally observed OH-CO complex to the HOCO intermediate." @default.
• W2080883335 created "2016-06-24" @default.
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• W2080883335 date "2001-01-01" @default.
• W2080883335 modified "2023-10-05" @default.
• W2080883335 title "Mapping the OH+CO→HOCO reaction pathway through IR spectroscopy of the OH–CO reactant complex" @default.
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• W2080883335 doi "https://doi.org/10.1039/b009421h" @default.
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