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• W2080914933 abstract "The time-resolved detection of excited-state vibrational motion and vibronic coupling with femtosecond pump-probe spectroscopy is analyzedwithin the framework of lowest-order perturbation theory with respect to the radiation-matter interaction. It is shown for the simple model of a shifted harmonic oscillator in the Condon approximation that coherent wave packet motion in the excited state is detectable with laser pulses of suitable duration (neither too long nor too short). It is furthermore shown that intramolecular coupling of an optically bright electronic state to a dark state via a single vibrational mode may lead to a pronounced oscillatory electronic population dynamics which can be detected in a pump-probe experiment with sufficiently short pulses. In both cases we analyze the conditions under which the phenomena manifest themselves in the time-resolved pump-probe signal." @default.
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• W2080914933 date "1988-08-01" @default.
• W2080914933 modified "2023-09-23" @default.
• W2080914933 title "Model studies on the time-resolved measurement of excited-state vibrational dynamics and vibronic coupling" @default.
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• W2080914933 doi "https://doi.org/10.1016/0301-0104(88)87152-0" @default.
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