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- W2080921981 abstract "The selective reduction of NO over Cu-, Co- and H-mordenite was studied using CH4, C2H4 and CH3OH, and compared with the same reaction in the gas phase. Co- and H-mordenite proved to be active and selective for the three reducing agents, while Cu-mordenite was so only when C2H4 and CH3OH were used. Besides being reduced in the presence of O2, NO acted as a homogeneous catalyst in the oxidation of CH4 and C2H4. A free-radical mechanism similar to the one occurring in the methane partial oxidation reaction could explain that behavior. Interestingly, on Co-mordenite, the conversion of nitric oxide to nitrogen began to occur at similar temperatures for both CH4 and CH3OH. For both Co-M and Cu-M the NO to N2 conversion started after the CH3OH conversion reached 100%. In the gas-phase reaction no NO conversion was observed when CH4 or C2H4 were used as reducing agents, but a 30% of the nitric oxide conversion was obtained when CH3OH was the reducing reactant at 600°C. Very similar results were observed with or without O2 in the feed stream. When catalysts were present, the presence of oxygen noticeably increased the rate of NO to N2 conversion." @default.
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- W2080921981 date "1995-12-01" @default.
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- W2080921981 title "On the role of gas-phase reactions in the mechanism of the selective reduction of NOx" @default.
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- W2080921981 doi "https://doi.org/10.1016/0926-3373(95)00032-1" @default.
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