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• W2080953606 startingPage "10083" @default.
• W2080953606 abstract "Electrochemical degradation on silicon (Si) anodes prevents them from being successfully used in lithium (Li)-ion battery full cells. Unlike the case of graphite anodes, the natural solid electrolyte interphase (SEI) films generated from carbonate electrolytes do not self-passivate on Si, causing continuous electrolyte decomposition and loss of Li ions. In this work, we aim at solving the issue of electrochemical degradation by fabricating artificial SEI films using a solid electrolyte material, lithium phosphorus oxynitride (Lipon), which conducts Li ions and blocks electrons. For Si anodes coated with Lipon of 50 nm or thicker, a significant effect is observed in suppressing electrolyte decomposition, while Lipon of thinner than 40 nm has a limited effect. Ionic and electronic conductivity measurements reveal that the artificial SEI is effective when it is a pure ionic conductor, but electrolyte decomposition is only partially suppressed when the artificial SEI is a mixed electronic-ionic conductor. The critical thickness for this transition in conducting behavior is found to be 40-50 nm. This work provides guidance for designing artificial SEI films for high-capacity Li-ion battery electrodes using solid electrolyte materials." @default.
• W2080953606 created "2016-06-24" @default.
• W2080953606 creator A5040315499 @default.
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• W2080953606 date "2014-06-19" @default.
• W2080953606 modified "2023-10-18" @default.
• W2080953606 title "Artificial Solid Electrolyte Interphase To Address the Electrochemical Degradation of Silicon Electrodes" @default.
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• W2080953606 doi "https://doi.org/10.1021/am5009419" @default.
• W2080953606 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/24926882" @default.
• W2080953606 hasPublicationYear "2014" @default.
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