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- W2081122141 abstract "The heavy fermion compound UPdIn is found to absorb deuterium without disproportionation to yield ${mathrm{UPdInD}}_{0.7}.$ Magnetization, heat capacity, x-ray, and neutron-diffraction measurements have been carried out to probe the structural and magnetic properties of this deuteride. It is found that deuterium absorption results in a highly anisotropic lattice expansion, without changing the ${mathrm{Fe}}_{2}mathrm{P}$-type hexagonal structure of the parent compound. The magnetic ordering temperature is enhanced to 80 K and the low-temperature uranium moment to $2.5{ensuremath{mu}}_{B}$ from their corresponding values of 21 K and $1.5{ensuremath{mu}}_{B},$ respectively, in the parent compound. Neutron-diffraction studies on the deuteride reveal antiferromagnetic ordering of the uranium moments and doubling of unit cell along the c axis. Heat capacity measurements show a large reduction in the value of electronic specific heat coefficient ensuremath{gamma} from 260 mJ ${mathrm{mol}}^{mathrm{ensuremath{-}}1}$ ${mathrm{K}}^{mathrm{ensuremath{-}}2}$ in UPdIn to 30 mJ ${mathrm{mol}}^{mathrm{ensuremath{-}}1}$ ${mathrm{K}}^{mathrm{ensuremath{-}}2}$ in ${mathrm{UPdInD}}_{0.7},$ indicating a significant reduction in the hybridization between uranium $5f$ electrons and those on the surrounding atoms." @default.
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- W2081122141 date "2002-12-31" @default.
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- W2081122141 title "Effect of deuterium absorption on the heavy-fermion compound UPdIn" @default.
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- W2081122141 doi "https://doi.org/10.1103/physrevb.66.214420" @default.
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