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• W2081189999 abstract "We report disorder to lamellar transition in a system of spherically symmetric particles where the interparticle potential consists of a short-ranged attraction and a longer-ranged repulsion. The system provides a simplified model for aqueous dispersions of colloidal particles and globular proteins that may exhibit stable/metastable clusters or microscopic phases. By using a non-mean-field density functional theory, we predict that under appropriate conditions, a lamellar phase with alternating condensed and dilute layers of particles is thermodynamically more stable than a uniform disordered phase at the same temperature and molecular number density. Formation of the lamellar structure may prohibit the macroscopic fluid-fluid phase transition. At a given condition, the width of the condensed lamellar layers increases with the overall particle density but the trend is opposite for the dilute lamellar layers. A minimal lamellar periodicity is obtained when the condensed and dilute layers have approximately the same thickness." @default.
• W2081189999 created "2016-06-24" @default.
• W2081189999 creator A5037660639 @default.
• W2081189999 creator A5088942752 @default.
• W2081189999 date "2009-04-23" @default.
• W2081189999 modified "2023-10-16" @default.
• W2081189999 title "Formation of lamellar structures from spherical particles" @default.
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• W2081189999 doi "https://doi.org/10.1063/1.3118681" @default.
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