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• W2081574712 abstract "Muon spin relaxation measurements in isotropic molecular magnets (MM) with a spin value $S$ ranging from $7/2$ to $27/2$ are used to determine the magnitude and origin of dephasing time ${ensuremath{tau}}_{ensuremath{phi}}$ of molecular magnets. It is found that ${ensuremath{tau}}_{ensuremath{phi}}ensuremath{sim}10text{ }text{ }mathrm{nsec}$ with no $S$ or ligand dependence. This indicates a nuclear origin for the stochastic field. Since ${ensuremath{tau}}_{ensuremath{phi}}$ is a property of the environment, we argue that it is a number common to similar types of MM. Therefore, ${ensuremath{tau}}_{ensuremath{phi}}$ is shorter than the Zener and tunneling times of anisotropic MM such as ${mathrm{Fe}}_{8}$ or ${mathrm{Mn}}_{4}$ for standard laboratory sweep rates. Our findings call for a stochastic Landau-Zener theory in this particular case." @default.
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• W2081574712 date "2007-06-22" @default.
• W2081574712 modified "2023-10-13" @default.
• W2081574712 title "Experimental Estimates of Dephasing Time in Molecular Magnets" @default.
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• W2081574712 doi "https://doi.org/10.1103/physrevlett.98.257204" @default.
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