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- W2081651789 abstract "Statistical thermodynamics is applied to available equilibrium hydrogen pressure-temperature-composition relationships for cubic hyperstoichiometric dihydrides, MH2+x (O < x < 1, M = La, Ce, Pr, Nd, Sm; Np, Pu, Am). A statistical model is constructed based on a perfect face centred cubic lattice of metal atoms with fully occupied tetrahedral interstitial sites by hydrogen atoms and partly and randomly occupied octahedral interstitial sites by the rest of hydrogen atoms. Atomic partition function of hydrogen in MH2+x is found to be similar for all MH2+x. On the other hand, the atomic partition function of metals in MH2+x for different M is found to be different. Mittels statistischer Thermodynamik werden verfügbare Gleichgewichtsbeziehungen: Wasserstoff-druck-Temperatur-Zusammensetzung für kubische hyperstöchiometrische Dihydride, MH2+x (O < x < 1, M = La, Ce, Pr, Nd, Sm, Np, Pu, Am) untersucht. Ein statistisches Modell wird konstruiert, das auf einem perfekten kubisch flächenzentrierten Gitter von Metallatomen mit vollständig besetzten tetraedrische Zwischengitterplätzen durch Wasserstoffatome sowie teilweise und statistisch besetzten Oktaederplätzen durch den Rest der Wasserstoffatome beruht. Es wird gefunden, daß die atomare Verteilungsfunktion von Wasserstoff in MH2+x für alle MH2+x ähnlich ist. Auf der anderen Seite wird gefunden, daß die atomare Verteilungsfunktion für Metalle in MH2+x für verschiedene M unterschiedlich ist." @default.
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- W2081651789 date "1983-08-01" @default.
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- W2081651789 title "Statistical Thermodynamic Approach to Some Hyperstoichiometric Dihydrides of Lanthanides (La, Ce, Pr, Nd, Sm) and Actinides (Np, Pu, Am)" @default.
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- W2081651789 doi "https://doi.org/10.1002/pssb.2221180238" @default.
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