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- W2081736002 abstract "Sodium cations solvated by polyethylene oxide have been confined by intercalation in the interlamellar space of an insulating layered solid, CdPS3. The frequency-dependent conductivity and the associated conductivity relaxation in the intercalated polymer electrolyte have been investigated. The temperature-dependent conductivity displays a distinct change in behavior at T∼225 K. Below 225 K the dc conductivity, σdc, shows an Arrhenius temperature dependence, while for T>225 K σdc rises sharply and follows the Vogel–Tamann–Fulcher relation, characteristic of ionic motion coupled to polymer relaxation modes. An analysis of the frequency-dependent conductivity using the electrical modulus representation showed that the electrical conductivity relaxation may be described in terms of the stretched exponential correlation function in the time domain, φ(t)=exp(−t/τσ)β. The absence of any anionic contribution to the electrical response makes these intercalated polymer electrolyte systems attractive for fundamental studies on ionic motion in disordered polymeric media." @default.
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- W2081736002 date "1998-11-08" @default.
- W2081736002 modified "2023-09-25" @default.
- W2081736002 title "Alternating current conductivity and electrical conductivity relaxation in an intercalated polymer electrolyte" @default.
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- W2081736002 doi "https://doi.org/10.1063/1.477458" @default.
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