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• W2081749346 abstract "We derive a self-similarity criterion that must hold if a planar electric double layer (EDL) can be captured by a local-density approximation (LDA), without specifying any specific LDA. Our procedure generates a similarity coordinate from EDL profiles (measured or computed), and all LDA EDL profiles for a given electrolyte must collapse onto a master curve when plotted against this similarity coordinate. Noncollapsing profiles imply the inability of any LDA theory to capture EDLs in that electrolyte. We demonstrate our approach with molecular simulations, which reveal dilute electrolytes to collapse onto a single curve, and semidilute ions to collapse onto curves specific to each electrolyte, except where size-induced correlations arise." @default.
• W2081749346 created "2016-06-24" @default.
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• W2081749346 date "2013-07-29" @default.
• W2081749346 modified "2023-10-18" @default.
• W2081749346 title "Model-free test of local-density mean-field behavior in electric double layers" @default.
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• W2081749346 doi "https://doi.org/10.1103/physreve.88.011301" @default.
• W2081749346 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/23944407" @default.
• W2081749346 hasPublicationYear "2013" @default.
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