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• W2081828005 abstract "Abstract A comparison has been made of the experimental and calculated relative values of the efficiency of capture by the acceptor molecule of an electron generated by ionizing radiations (the α coefficient in Hummel's theory) in liquid hydrocarbons at room temperature; pentadecane, n -hexane, iso-octane and neopentane. For the experimental determination of the values of α the authors used the measurements of luminescence induced by a pulse of fast electrons in solutions of pyrene (10 15 −10 16 cm −3 ) in hydrocarbons. Calculation of the values of α for the diffusion description of the process of recombination of an electron is based on the relation: α ≈ K S r m 3/ u , where K S is the rate constant of capture of an electron by the molecule of pyrene; u is the drift mobility of the electron; r m is the most probable distance of thermolysation of an electron. The values of K S and u for pentadecane and neopentane were determined by investigation of the electrical conductivity induced by a pulse of fast electrons in solutions of pyrene; for K S and u in the case of n -hexane and iso-octane and also for r m the published data were used. It is shown that while for hydrocarbons with relatively low mobility of the electron the calculated and experimental values of α agree, for the hydrocarbon with the highest mobility of the electron (neopentane) use of diffusion concepts for the calculation gives an overstated value of α." @default.
• W2081828005 created "2016-06-24" @default.
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• W2081828005 date "1976-01-01" @default.
• W2081828005 modified "2023-09-25" @default.
• W2081828005 title "The validity of diffusion concepts for describing the kinetics of recombination of an excess electron in liquid hydrocarbons" @default.
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• W2081828005 doi "https://doi.org/10.1016/0020-7055(76)90015-2" @default.
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