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- W2081856310 abstract "Advanced reburning technology, which makes use of natural gas injection followed by ammonia injection, has proven to be an effective method for the removal of up to 85−95% of the NO in pulverized, coal-fired furnaces. This paper reports the development of a seven-step, 11-species reduced mechanism for the prediction of nitric oxide concentrations using advanced reburning from a 312-step, 50-species full mechanism. The derivation of the reduced mechanism is described, including the selection of the full mechanism, the development of the skeletal mechanism, and the selection of steady-state species. The predictions of the seven-step reduced mechanism are in good agreement with those of the full mechanism over a wide range of parameters, applicable to coal-based, gas-based, and oil-based combustion cases. Comparisons with three independent sets of experimental laminar data indicate that the reduced mechanism correctly predicts the observed trends, including the effects of temperature, the ratio of (NH3/NO)in, and concentrations of CO, CO2, O2, and H2O on NO reduction. The observed effects of CO on NH3 slip were also reliably predicted. Mechanistic considerations provide an explanation for the roles of the important radicals and species. Also, parametric studies of the effects of CO2 and H2O have been performed with the reduced mechanism. A maximum in NO reduction exists, which strongly depends on the concentrations of NOin, CO, and O2, the ratio of (NH3/NO)in, and temperature." @default.
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- W2081856310 date "1998-10-17" @default.
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- W2081856310 title "A Reduced Kinetic Model for NO<i><sub>x</sub></i> Reduction by Advanced Reburning" @default.
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- W2081856310 doi "https://doi.org/10.1021/ef980084l" @default.
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