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• W2082480147 abstract "Experimental and detailed chemical kinetic modeling has been performed to investigate aromatic and polycyclic aromatic hydrocarbon formation pathways in a premixed, rich, sooting, ethylene-oxygen-argon burner stabilized flame. An atmospheric pressure, laminar flat flame operated at an equivalence ratio of 3.06 was used to acquire experimental data for model validation. Gas composition analysis was conducted by an on-line gas chromatograph/mass spectrometer (GC/MS) technique. Measurements were made in the flame and postflame zone for a number of low molecular weight species, aliphatics, aromatics, and polycyclic aromatic hydrocarbons (PAHs) ranging from two-to five-fused aromatic rings. The modeling results show that the key reaction sequences leading to aromatic and polycyclic aromatic hydrocarbon growth involve the combination of resonantly stabilized radicals. In particular, propargyl and 1-methylallenyl combination reactions lead to benzene and methyl-substituted benzene formation, while polycyclic aromatics are formed from cyclopentadienyl radicals and fused rings that have a shared C5 side structure. Naphthalene production through the reaction step of cyclopentadienyl self-combination and phenanthrene formation from indenyl and cyclopentadienyl combination were shown to be important in the flame-modeling study. The removal of phenyl by O2 leading to cyclopentadienyl formation is expected to play a pivotal role in the PAH or soot precursor growth process under fuel-rich oxidation conditions." @default.
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• W2082480147 date "1996-01-01" @default.
• W2082480147 modified "2023-10-11" @default.
• W2082480147 title "Experimental and modeling investigation of aromatic and polycyclic aromatic hydrocarbon formation in a premixed ethylene flame" @default.
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• W2082480147 doi "https://doi.org/10.1016/s0082-0784(96)80277-3" @default.
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