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- W2082530460 abstract "The thermodynamic properties of the transporting reactions in the closed-tube ZnSe−N−H−Cl system are analyzed by solving a set of equations with numerical methods, where NH4Cl serves as the transport agent. The results show that ZnSe−NH4Cl system has the properties of high total pressure and low transporting reaction equilibrium constant. The decomposition of hydrogen selenide determines the difference between the partial pressures of ZnCl2 and H2Se, which slows down the growth rate. This difference can be adjusted by adding extra Se and the hydrogen (H2) produced through decomposition of NH3. The ZnCl2 and a little extra Se should be added into the ZnSe−NH4Cl system to improve the utilizing efficiency of H2 and the concentration of practical transporting components of ZnCl2 and H2Se. A ZnSe single crystal as large as 20 × 15 × 8 mm3 was obtained by using ZnCl2·2NH4Cl as the transport agent with a little extra Se at about 1300 K. The experimental results about the diffusion-limited transport rate are well coincided to the thermodynamical analysis." @default.
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- W2082530460 date "2008-09-06" @default.
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- W2082530460 title "Thermodynamic Analysis and Single Crystal Growth of ZnSe from ZnSe−N−H−Cl System" @default.
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- W2082530460 doi "https://doi.org/10.1021/cg070337d" @default.
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