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• W2082660219 abstract "High-performance liquid chromatography was used to isolate two new trimetallic nitride endohedral fullerenes, Gd3N@C2n (n = 42 and 44), and they were characterized by MALDI-TOF mass spectrometry, UV−vis−NIR, and cyclic voltammetry. It was found that their electronic HOMO−LUMO gaps depend pronouncedly on the size of the cage, from a large band gap for Gd3N@C80 (2.02 V) to a small band gap for Gd3N@C88 (1.49 V). The electrochemical properties also change dramatically with the size of the cage, going from irreversible for the C80 cage to reversible for Gd3N@C88. The latter is the largest trimetallic cluster inside C88 isolated and characterized to date. Gd3N@C88 has one of the lowest electrochemical energy gaps for a nonderivatized metallofullerene." @default.
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• W2082660219 date "2007-11-06" @default.
• W2082660219 modified "2023-10-11" @default.
• W2082660219 title "Gd₃N@C₂<i>_n</i> (<i>n</i> = 40, 42, and 44): Remarkably Low HOMO−LUMO Gap and Unusual Electrochemical Reversibility of Gd₃N@C₈₈" @default.
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• W2082660219 doi "https://doi.org/10.1021/ja075930y" @default.
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