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- W2082741827 abstract "Abstract The crystal structures and physical properties of molecular magnets developed in our group are reviewed. (1) (DMET)2FeBr4 and its analogues are composed of alternating stacks of quasi-one-dimensional donor sheets and square lattice magnetic anion sheets. These salts undergo an SDW transition of the donor layer and an antiferromagnetic transition of Fe3+ spins on the anion layer. The one-to-one correspondence of the anomalies appearing on the magnetization curves and the magnetoresistance supports the presence of the π–d interaction. On applying pressure, a large negative magnetoresistance is observed for the all-sulfur compound (EDTDM)2FeBr4 in the marginal region of the SDW and metallic ground states. (2) (BDH-TTP)[M(isoq)2(NCS)4] (M=Cr, Fe) show bulk weak ferromagnetism at 7.6 K. The donor cation radicals (S=1/2) and anions (S=3/2 (Cr), 5/2 (Fe)) form ferrimagnetic chains with close intermolecular S⋯S contacts, which are then antiferromagnetically coupled through the π–π overlap of the ligands and inter-chain S⋯S contacts of the donors. The non-collinear alignment of the molecular axes of adjacent anions is responsible for the canted spin structure." @default.
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- W2082741827 date "2003-07-01" @default.
- W2082741827 modified "2023-10-18" @default.
- W2082741827 title "π–d Interaction-based molecular magnets" @default.
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- W2082741827 doi "https://doi.org/10.1016/s0277-5387(03)00178-5" @default.
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