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- W2082772076 abstract "The T←N (π→π*) transitions in ethylene, all of its methyl derivatives, and 1-butene were observed by means of He+-impact energy-loss spectroscopy. With a resolution of better than 0.1 eV, a vibrational structure was just resolved in the T←N excitation spectrum of ethylene. The T←N transition energy was measured for the alkylethylenes with a lower resolution. The results are in good agreement with the electron-impact data, indicating that the vibro-rotational excitation due to the impulsive momentum transfer is negligible in the present method. The T←N excitation cross-sections were found to decrease by half upon the unit substitution of alkyls. The relative invariance of the T←N transition energy and the decrease in the T←N cross-sections upon alkyl substitution may be attributable to the decrease in the intra- and intermolecular Coulomb and exchange interactions between π- and π*-orbitals." @default.
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- W2082772076 date "1982-04-01" @default.
- W2082772076 modified "2023-09-23" @default.
- W2082772076 title "An Ion-impact Study of Singlet-Triplet Transitions in Ethylene and Alkyl-substituted Ethylenes" @default.
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- W2082772076 doi "https://doi.org/10.1246/bcsj.55.1290" @default.
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