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• W2083466929 endingPage "9413" @default.
• W2083466929 startingPage "9402" @default.
• W2083466929 abstract "The low-temperature rotational relaxation of CO in self-collisions and in collisions with the rare-gas atoms Ne and He has been investigated in supersonic expansions with a combination of resonance-enhanced multiphoton ionization (REMPI) spectroscopy and time-of-flight techniques. For the REMPI detection of CO, a novel 2 + 1‘ scheme has been employed through the A1Π state of CO. From the measured data, average cross sections for rotational relaxation have been derived as a function of temperature in the range 5−100 K. For CO−Ne and CO−He, the relaxation cross sections grow, respectively, from values of ∼20 and 7 Å2 at 100 K to values of ∼65−70 and ∼20 Å2 in the 5−20 K temperature range. The cross section for the relaxation of CO−CO grows from a value close to 40 Å2 at 100 K to a maximum of 60 Å2 at 20 K and then decreases again to 40 Å2 at 5 K. These results are qualitatively similar to those obtained previously with the same technique for N2−N2, N2−Ne, and N2−He collisions, although in the low-temperature range (T < 20 K) the CO relaxation cross sections are significantly larger than those for N2. Some discrepancies have been found between the present relaxation cross sections for CO−CO and CO−He and the values derived from electron-induced fluorescence experiments." @default.
• W2083466929 created "2016-06-24" @default.
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• W2083466929 date "2005-09-29" @default.
• W2083466929 modified "2023-10-18" @default.
• W2083466929 title "Low-Temperature Rotational Relaxation of CO in Self-Collisions and in Collisions with Ne and He" @default.
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• W2083466929 doi "https://doi.org/10.1021/jp051766u" @default.
• W2083466929 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/16866388" @default.
• W2083466929 hasPublicationYear "2005" @default.
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