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• W2083554748 abstract "Spectrophotometric and electrochemical investigations have shown that the bis(2,2′-bipyridine)(2-(2′-pyridyl)-benzimidazole)ruthenium(II) cation and its derivatives interact with aromatic nitrogen heterocycles (N-heterocycles) through hydrogen bonding. The equilibrium constant for the hydrogen bonding was increased with increasing pKa value of the N-heterocycles. The Ru(II/III) oxidation potential, E12, was shifted cathodically by 200–400 mV due to the hydrogen bonding interaction. The magnitude of this potential shift shows the linear dependence on the base strength pKa of the N-hetero-cycles. The hydrogen bonding interaction for the Ru(III) oxidation state was found to be much stronger than that for the Ru(II) state. We suggest the potential use of the present Ru-benzimidazole and -imidazole complexes as a spectrophotometric and electrochemical probe for examining the micro-environment in biopolymers." @default.
• W2083554748 created "2016-06-24" @default.
• W2083554748 creator A5053601852 @default.
• W2083554748 creator A5081293252 @default.
• W2083554748 date "1989-10-01" @default.
• W2083554748 modified "2023-09-23" @default.
• W2083554748 title "The outer-sphere interactions in ruthenium and osmium complexes I. Spectrophotometric and voltammetric studies on the hydrogen bonding interactions of bis(2,2′-bipyridine)(2-(2′-pyridyl)-benzimidazole)ruthenium(II)cation and its derivatives with aromatic nitrogen heterocycles" @default.
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• W2083554748 doi "https://doi.org/10.1016/s0020-1693(00)83214-4" @default.
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