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• W2083657300 abstract "Inelastic neutron scattering experiments have been carried out on expanded liquid rubidium in a density range between the melting point density and about twice the critical density. The dynamics of the liquid show metallic-like behavior even at relatively low densities. In expanding the liquid further to about twice the critical density, where a breakdown of the metallic properties is expected, S(Q, ω) changes its shape considerably. It is now characterized by a localized excitation, indicating that molecules present in the dilute vapour may survive the condensation into the dense fluid. First principles total energy calculations for Rb-lattices at 0 K support this view and predict that expansion favours spin pairing leading to the formation of Rb2 molecules with a continuous increase in vibron energy with decreasing density. Excellent agreement is found between the calculated vibron energy and the experimental result." @default.
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• W2083657300 date "1997-12-01" @default.
• W2083657300 modified "2023-09-28" @default.
• W2083657300 title "The formation of a molecular state in expanded liquid rubidium" @default.
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• W2083657300 doi "https://doi.org/10.1016/s0921-4526(97)00757-6" @default.
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