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• W2083663301 startingPage "2546" @default.
• W2083663301 abstract "We show, by carefully examining the change of total energy in constrained variational calculations using the local spin density approximation, that crystal field excitations in normal rare earths are quasiparticles composed of a $4f$ excitation plus its associated cloud of shielding conduction electrons. Total energy calculations, which properly exclude the self-interaction of the nonspherical part of the $4f$ densities, are then used to calculate crystal field energies and the corresponding spin Hamiltonian parameters of TmSb and PrSb, accurately from first principles." @default.
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• W2083663301 date "1997-09-29" @default.
• W2083663301 modified "2023-09-24" @default.
• W2083663301 title "Density Functional Theory of Crystal Field Quasiparticle Excitations and the<i>Ab Initio</i>Calculation of Spin Hamiltonian Parameters" @default.
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• W2083663301 doi "https://doi.org/10.1103/physrevlett.79.2546" @default.
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