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• W2083706677 abstract "Electronic excitations in linear chains and icosahedra clusters of gold atoms have been studied using an approximate version of time-dependent density functional theory based on the extended Hückel tight-binding method. The formation and development of two longitudinal collective resonances in the absorption spectra were studied as a function of the chain length. We show that in the case of a gold cluster dimer, the classical description breaks down at intercluster distances below 0.5 nm due to the neglect of important quantum effects. In addition, a blue shifting of the collective resonances at these distances is observed. Analysis of these results yields a general picture of electronic resonances in one-dimensional atomic structures." @default.
• W2083706677 created "2016-06-24" @default.
• W2083706677 creator A5018058115 @default.
• W2083706677 creator A5062566652 @default.
• W2083706677 date "2010-11-15" @default.
• W2083706677 modified "2023-10-16" @default.
• W2083706677 title "Extended Hückel Tight-Binding Calculations of Electronic Resonances in Linear Chains of Gold Atoms and Clusters" @default.
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• W2083706677 doi "https://doi.org/10.1021/jp106761f" @default.
• W2083706677 hasPublicationYear "2010" @default.
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