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- W2083727299 abstract "Soft-x-ray photoemission and absorption spectroscopies are employed to investigate the electronic structures of ${text{Sr}}_{1ensuremath{-}x}{text{Rh}}_{2}{text{O}}_{4}$. Similar to the layered cobaltates such as ${text{Na}}_{1ensuremath{-}x}{text{CoO}}_{2}$, a valence-band satellite feature (VBS) occurs at higher binding energy to the $text{O}text{ }2p$ band. We find that the VBS resonates at the $text{O}text{ }1s$ edge. Additionally, core absorption shows clear $x$ dependence in the $text{O}text{ }1s$ edge rather than in the $text{Rh}text{ }3p$ edge. These results indicate that the holes in the initial state mainly have $text{O}text{ }2p$ character presumably due to $dtext{ensuremath{-}}p$ rehybridizations affected by ${text{Sr}}^{2+}$ vacancy potentials. The resultant inhomogeneous charge texture may have impact on the thermoelectric transport properties at low $x$." @default.
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- W2083727299 date "2009-08-12" @default.
- W2083727299 modified "2023-10-02" @default.
- W2083727299 title "Evidence for oxygen holes due to<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:mi>d</mml:mi><mml:mtext>−</mml:mtext><mml:mi>p</mml:mi></mml:mrow></mml:math>rehybridization in thermoelectric<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:msub><mml:mrow><mml:mtext>Sr</mml:mtext></mml:mrow><mml:mrow><mml:mn>1</mml:mn><mml:mo>−</mml:mo><mml:mi>x</mml:mi></mml:mrow></mml:msub><mml:msub><mml:mrow><mml:mtext>Rh</mml:…" @default.
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- W2083727299 doi "https://doi.org/10.1103/physrevb.80.081103" @default.
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